The documents acknowledge that the duo had an "informal arrangement", but that Pitt has not lived up to that agreement.
Meanwhile, Jolie is also urging the judge to issue a final divorce decree this year to legally restore her single status, reports TMZ.
According to new court documents obtained by "Good Morning America", the actress is seeking formal child support from her estranged husband, claiming he has not financially contributed in a "meaningful" way to their six children's well-being since their 2016 separation.
"Respondent has a statutory duty to pay child support".
The declarations came in a request for a case-management hearing filed Tuesday by Jolie Pitt's attorneys in Los Angeles Superior Court.
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"Given the informal arrangements around the payment of the children's expenses have not been regularly sustained by [Pitt] for over a year and a half".
The increasingly bitter battle between the two movie stars has focused around the parenting and custody of their children - Maddox, 16, Pax, 14, Zahara, 13, Shiloh, 12, and 10-year-old twins Vivienne and Knox.
The brood is now living in London with Jolie as she films Maleficent 2, while Pitt has spent his court-ordered time with the kids in London and Los Angeles, where he is shooting Quentin Tarantino's new movie, Once Upon a Time in Hollywood. "The motion today was just created to move that process forward on those issues, including financial disclosure and child support", a source close to Jolie explained to E!
The drama in the long-running divorce case of former Hollywood power couple Angelina Jolie and Brad Pitt has hit a new level.
FILE PHOTO: Cast member Brad Pitt and actress Angelina Jolie pose at the premiere of "The Tree of Life" at LACMA in Los Angeles, California, U.S., May 24, 2011.